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It is probable, however, that the mechanism is # morc complicated than just a single elementary bimolccular reaction. Reutov and coworker^'"^ have studied rcaction 41 (R = PhCH,; R = CF,, CCI,; X = CI, I, OCOCF,). They showed that the reaction was first order with respect to each reactant and obtained second-order rate constants in a variety of solvents (Table 16). For this set of reactions, a cyclic transition state was proposed'"'. - T A B L E 16. 0005 46 Michael H. Abraham and Priscilla L. Grellier Jcnscn and Miller"'* reported that the thrcc-alkyl exchange 42 occurred almost instantaneously, with precipitation of PhHgBr, but that the subscqucnt three-alkyl exchange 43 took place much more slowly.

J. Pickett I n conclusion, electrochemical metnl--carbon ligand bond cleavage reactions and related ligand centred electrochemistry still hold considerable promise for the futurc. VI. ACKNOWLEDGEMENTS I thank Dr D. R. Stanley for reading the manuscript and for h e l p f u l comments. VII. REFERENCES 1. R. N. Adams, Electrocliernistry at Solid Electrodes, Marcel Dekker, New York, 1969. 2. D. T. Sawyer and J. L. Roberts, Experinieritd Electroclrettiistry for Chemists, Wiley, New York, 1974. 3. D.

Besenhard, A. Frank and D. Neugebauer, J. Organornet. , 191,261 (1980). 90. R. Riedce, H. Kofima, and K. Oelfele, Angew. , 92, 550 (1980). 91. A. Bell, D. D. Klendworth, R. E. Wild, and R. A. Walton, Inorg. , 20,4457 (1981). 92. P. Lemoinc and M. Gross, C. R. Acad. , Ser. C, 280,797 (1975). 93. P. Lernoine and M. Gross, Electrochim. Acta, 1, 121 (1976). 94. N. El Murr and A. Chaloyard, Inorg. , 21, 2206 (1982). 95. A. M. Bond, R. Colton, and J. J. Jackowski, Inorg. , 14, 174 (1975). 96. C. J. Pickett and D.

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